Catalytic Transfer Functionalization through Shuttle Catalysis

Catalytic Transfer Functionalization through Shuttle Catalysis

Catalytic Transfer Functionalizat ion through Shuttle Catalysis Bhawal, Benjamin N., Bill Morandi. ACS Catalysis, 2016, 7528-7535. 1. Shuttle Catalysis Concept

2. Selected Examples of Shuttle Catalysis Reactions 3. Summary 1. Shuttle Catalysis Concept

2. Scheme 1. Transfer Hydrogenation

2. 1. Wang, Dong, Didier Astruc. Chemical reviews , 2015, 6621-6686. Scheme 2. Generalization of the Shuttle Catalysis Concept

Scheme 3. Definition of Forward and Reverse Shuttle Catalysis Reaction 2. Selected Examples of Shuttle Catalysis Reactions

Scheme 4. MetalOrganic Cooperatively Catalyzed Hydroacylation of Alkenes by Transfer of an Aldehyde 2. Jun, C.-H.; Lee, H. J. Am. Chem. Soc. 1999, 121, 880881.

Scheme 5. Rhodium-Catalyzed Retro-hydroformylation of Aldehydes 3. Murphy, S. K.; Park, J.-W.; Cruz, F. A.; Dong, V. M. Science. 2015, 347, 5660. Scheme 6. Alkene Transfer Hydrocyanation, the Forward Process

4. Fang, X.; Yu, P.; Morandi, B. Science 2016, 351, 832836. Scheme 7. Retro-hydrocyanation, the Reverse Process 5. Lo, J. C.; Yabe, Y.; Baran, P. S. J. Am. Chem. Soc. 2014, 136, 13041307.

Scheme 8. Catalytic Transfer Hydromagnesiation 6. Shirakawa, E.; Ikeda, D.; Masui, S.; Yoshida, M.; Hayashi, T. J. Am. Chem. Soc. 2012, 134, 272279.6.

Scheme 9. Catalytic Transfer Silacyclopropanation 7. Driver, T. G.; Woerpel, K. A. J. Am. Chem. Soc. 2003, 125, 1065910663. 1.

2. 3.

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